What are helpful "extra" recordings for Chinese?

Nohkara

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Yo!

I've plans to record a simple "CV style" Voice Bank for Chinese:

From what I know so far is that a minimum amount of "syllable" what you need for Chinese is reading around those 400 different Pinyin combinations but are there any "syllable" that are outside that chart
(e.g. "ki" or "kya" aren't in Chinese Pinyin from what I know) but are still actually "pronounceable" and "useful" for example for Chinglish.

I'm 99,9% sure that Chinese Vocaloids has some extra recordings that aren't in Pinyin chart, so I'm looking for extra recordings like that(?)

Obviously, I won't record "all C+V combinations" because that would be too time taking plus basic Chinese has all ready around 400 syllables and it's just... pointless for Chinese if I done all, so try name just "few" that can be actually somehow useful ones. Thanks!
 

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